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Hi Ralf,
In the Time Slices window, one full day runs from the beginning of 'hour 0' to the beginning of 'hour 24' (so, 24 hours in total). Weeks run from Monday through the following Sunday (seven days in total), only because LEAP lists weekdays before weekends (rather than a week starting on Sunday, as you see in many wall calendars, it starts on Monday).
The time slices that you're trying to create do in fact require a bit more massaging in order to build into LEAP. Even the detailed setup options, under General:Time Slices, don't quite give you the amount of flexibility that you need. You'll have to build the time slices you want outside of LEAP, but in a way that they can be imported.
My advice would be to use LEAP's time slices setup tool in the same way that you have, but then export the slices to Excel. That way you'll be able to modify them without interrupting the formatting. One you're done tinkering, use the Import button in the Time Slices window to pull them back into LEAP.
I've gone ahead and started this, so you know what I mean. You can find a sample file here:
ftp://forums.seib.org/areas2012/sample_time_slices.xlsx
NB: At least for the time being - again, we're working to address this - there is a small problem with the way LEAP allocates load data to each of the hourly slices, in the Yearly Shapes screen. After properly setting your time slices, and then importing a yearly shape, you may find that for the time slice corresponding to hour 0 - 1 the percentage of annual energy load is 2X what it should be, yet the time slices from hour 23 - 24 contains no data. You will have to manually edit the curve for these two time slices.
Regarding the computational effort needed to resolve hourly time slice data, I think you should be okay here. You're still only considering 192 slices per year (rather than 8760, if you wanted to resolve each hour individually). The computational time will probably be more affected by the number of scenarios that you're running, and the number of years in these scenarios.
Good luck,
Taylor