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Hi Sultan,
At some point, you will need to identify the saturation (or shares) of each fuel in the input energy mixture for each of your industries - this is important. These fuel saturations may be '100%' (meaning that each fuel is required for every unit of industrial output), but you'll need to make that assumption.
Industrial production of each fuel is less of a concern, since if the fuel is not produced in the region, you can always set LEAP to import it.
This hints at one of the issues you will come across while conducting regional modeling, from my own experience (although I am unable to provide you with a LEAP example). Many of the fuels consumed in the embedded region may me imported from the larger region, and conversely, some of the fuels generated in Basque Country (i.e. any electricity generation) may not necessarily be consumed there.
When doing your demand modeling you may also find that conducting a simple, national-level model helps you to fill in gaps, for which you have difficulty finding data specific to Basque Country itself.
You mentioned only industrial demand - but have you thought about other sectors (commercial or agricultural, as well as household demand and transportation)?
You may also find the following link useful - this is a starter document intended to address many different data requirements, but it will help guide your data collection nonetheless:
www.energycommunity.org/uploads/LEAP_Data_Requirements.doc
Hope this helps,
Taylor